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Yellowing of leaves with green veins could be iron deficiency and/or high soil pH. If on top of this yellowing, the leaves are also smaller than normal then it could also be a zinc deficiency. I would check soil pH first.
based on pics here-https://www.permablitz.net/articles/identifying-plant-nutrient-deficiencies/I'd guess Iron Potassium or MagnesiumHave you done a soil or leaf test?
Not sure but a pH of 6.8 could be on the higher end for Langsat. I believe where it originates, the pH is around 6 on average.
The only sure way I know is what you already put in place, sulfur pellets. Maybe add more of it and less watering which could wash away the sulfur (?).Another thing I could think of would be to spray something like this "Fertilome (10630) Chelated Liquid Iron and Other Micronutrients", if lowering pH is too hard. I use this for drenching but spray should do as well.
Looks like Mg maybe induced by excessive use of an antagonistic macro like Ca. Maybe other nutrients in deficiency or excess I have a few trees. PH of 5.5 to about 7.5 should be ok but winter mins below 7c can cause distress